modified on 28 July 2015 at 14:11 ••• 7,112 views


From Sanli Faez

Jump to: navigation, search

Resonant coupling to single molecules in nanoguides

A few decades ago, studying single quantum emitters such as atoms, ions, or molecules was a dream, but today such investigations have become commonplace in many laboratories. Building on the fantastic ingredients of the single-emitter physics toolbox, many scientists now wish to realize mesoscopic ensembles made of carefully-arranged individual quantum entities that are interconnected by quantum messengers such as visible photons. Such a network is sometimes called a quantum web. However, the direct photonic coupling of two emitters placed at distances larger than a wavelength is usually negligible. To enhance this interaction, one might use high-finesse cavities and although the first steps have been taken, it remains a very challenging experiment with severe limitations on its prospects for scalability to many atoms. An alternative approach for efficient light-matter interaction has been shown to involve tight focusing of propagating photons, but this strategy is also difficult to scale to a large number of emitters.

At the Max-Planck Institute for the Science of Light in Erlangen, we built an efficient solid-state platform for coherent interaction between photons and single molecules. Our system consists of organic dye molecules embedded inside an organic crystal that fills a glass nanocapillary to form an optical waveguide with a sub-wavelength mode diameter. With a careful choice of materials and fabrication process, each dye molecule acts like a quantum two-level system with a very high degree of coherence. We have measured the transmission of photons through this nanoguide and have seen that each time the frequency of the laser beam matches the narrow optical transitions of the individual molecules, there is an extinction signal of a few percent. Because the interaction between each molecule and light takes place via elastic scattering, the quantum coherence is preserved. The results were published in Physical Review Letters (Vol. 113, No. 213601).

Observation of Multifractality at the Anderson transition of ultrasound

Waves usually diffuse through random materials. This fact allows light to travel through thick clouds and electrons to conduct through metals. But disorder can sometimes bring wave propagation to a complete halt. This remarkable phase transition from conductor to insulator, suggested by Philip Anderson in 1958, is known as Anderson localization. Ad and I, together with John Page and Anatoliy Strybulevych from Manitoba, Canada, and Bart van Tiggelen from Grenoble have uncovered the essential structure of waves close to the transition point. We studied ultrasound propagation in a disordered network of aluminum beads. Just below the Anderson transition threshold wildly fluctuating forked wave-patterns, so-called multifractals, arise. The observation of multifractality in waves finally brings theories of the structure of the localization transition developed over the last 25 years, face to face with reality. The Anderson localization transition, once such an out-of-reach complex theory that Philip Anderson called his seminal paper "the unrecognizable monster" in his 1977 Nobel prize lecture, has evolved into a sub-branch of condensed matter theory with applications found in electronic conductivity of solids, transport of light and sound in multiple-scattering media, the quantum hall transition, high-T_c superconductivity, and the conductivity of Graphene. In fact, the concept of multifractality extends beyond localization. Multifractals are found in many complex systems such as turbulence, earthquakes, and patterns of rainfall.

Development of Refractive Index Tuning method

Measuring how fast light energy travels is not so easy, but inside opaque materials, like clouds, bone, skin, or paint the problem is particularly hairy. We have teased out this rate of transport using a simple, yet novel, trick: changing the ambient pressure. As the pressure is slowly tuned so is the so-called effective refractive index, which determines the speed of light. Even though the light is following an extremely complex path as it bounces through the material, its speed can be characterized by tracking the influence of pressure on the outgoing light intensity pattern. So simple and direct is the technique that it offers an entirely new way for probing inside important biological materials such as bone or wood as well as complex photonic materials such as photonic crystals or metamaterials. Our letter on this subject is published in Physical Review Letters (Vol. 103, No. 053903). ScienceNews Magazine has also publicized this work here.